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141.
Ambient afterglow luminescence from metal‐free organic chromophores would provide a promising alternative to the well‐explored inorganic phosphors. However, the realization of air‐stable and solution‐processable organic afterglow systems with long‐lived triplet or singlet states remains a formidable challenge. In the present study, a delayed sensitization of the singlet state of organic dyes via phosphorescence energy transfer from organic phosphors is proposed as an alternative strategy to realize “afterglow fluorescence”. This concept is demonstrated with a long‐lived phosphor as the energy donor and commercially available fluorescent dyes as the energy acceptor. Triplet‐to‐singlet Förster‐resonance energy‐transfer (TS‐FRET) between donor and acceptor chromophores, which are co‐organized in an amorphous polymer matrix, results in tuneable yellow and red afterglow from the fluorescent acceptors. Moreover, these afterglow fluorescent hybrids are highly solution‐processable and show excellent air‐stability with good quantum yields. 相似文献
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Suman Kuila Prof. Dr. Subi J. George 《Angewandte Chemie (Weinheim an der Bergstrasse, Germany)》2020,132(24):9479-9483
Ambient afterglow luminescence from metal-free organic chromophores would provide a promising alternative to the well-explored inorganic phosphors. However, the realization of air-stable and solution-processable organic afterglow systems with long-lived triplet or singlet states remains a formidable challenge. In the present study, a delayed sensitization of the singlet state of organic dyes via phosphorescence energy transfer from organic phosphors is proposed as an alternative strategy to realize “afterglow fluorescence”. This concept is demonstrated with a long-lived phosphor as the energy donor and commercially available fluorescent dyes as the energy acceptor. Triplet-to-singlet Förster-resonance energy-transfer (TS-FRET) between donor and acceptor chromophores, which are co-organized in an amorphous polymer matrix, results in tuneable yellow and red afterglow from the fluorescent acceptors. Moreover, these afterglow fluorescent hybrids are highly solution-processable and show excellent air-stability with good quantum yields. 相似文献
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采用高温固相法制备了Y2O2S ∶ Eu,Mg,Ti,Gd红色长余辉材料,研究了热处理工艺对材料稳定性的影响。用X射线衍射表征该材料的相组成,用激发光谱、发射光谱、余辉亮度对材料的发光性能进行表征。结果表明:热处理温度在600 ℃以下时,材料的发光性能不变;当热处理温度达到800 ℃时,发光性能缓慢下降;当热处理温度达到1 000 ℃时,主晶相Y2O2S变成Y2O2SO4和Y2O3,发光性能急剧下降。与铝酸盐及硫化物发光材料相比,Y2O2S ∶ Eu,Mg,Ti,Gd红色长余辉材料具有较好的热稳定性。 相似文献
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Development of afterglow time test system for nanosecond fluorescent screen of low-level-light image intensifier北大核心CSCD 下载免费PDF全文
The time characteristics of fluorescent screen is one of the important parameters to evaluate the performance of image intensifier. At present, there is no measurement method for the afterglow time of nanosecond fluorescent screen of low-level-light image intensifier. Based on the traditional test scheme of image intensifier afterglow time, a afterglow time test system for nanosecond fluorescent screen was developed. This system used a high-speed signal generator with the sampling rate of 250 MHz to complete the excitation of the laser diode light pulse, and a photomultiplier tube was used with the descending time of 0.57 ns to complete the photoelectric conversion of the fluorescent screen light signal. The weak photocurrent signal of μA magnitude was amplified and converted to a single-terminal differential circuit to complete the AD conversion in AD9684. Then the digital luminance information of the fluorescent screen was stored in the double data rate SDRAM (DDR) unit after field programmable gate array (FPGA), and the host computer sent instructions to read the DDR memory. The USB3.0 high-speed transmission protocol was used to transmit data to the host computer. In the data processing, the Kalman filtering and fast finding falling edge algorithm were used to realize the accurate measurement of noise filtering from collected data and afterglow time. The test results show that the proposed afterglow time test system for nanosecond fluorescent screen can effectively test the image intensifier with ultrafast optical characteristics. The afterglow test results of P47 phosphor reaches 118.094 4 ns, and the repeatability reaches 2.08%. © 2022 Editorial office of Journal of Applied Optics. All rights reserved. 相似文献
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